Investigation of carbon nanotube growth termination mechanism by in-situ transmission electron microscopy approaches

Title
Investigation of carbon nanotube growth termination mechanism by in-situ transmission electron microscopy approaches
Authors
김승민정서정김환철
Keywords
in-situ TEM; in-situ CNT growth; CNT growth termination mechanism; carbon nanotubes; growth termination; catalyst morphology; in-situ transmission electron microscope; tip growth mode
Issue Date
2013-10
Publisher
Carbon Letters
Citation
VOL 14, NO 4, 228-233
Abstract
In this work, we report in-situ observations of changes in catalyst morphology, and of growth termination of individual carbon nanotubes (CNTs), by complete loss of the catalyst particle attached to it. The observations strongly support the growth-termination mechanism of CNT forests or carpets by dynamic morphological evolution of catalyst particles induced by Ostwald ripening, and sub-surface diffusion. We show that in the tip-growth mode, as well as in the base-growth mode, the growth termination of CNT by dissolution of catalyst particles is plausible. This may allow the growth termination mechanism by evolution of catalyst morphology to be applicable to not only CNT forest growth, but also to other growth methods (for example, floating-catalyst chemical vapor deposition), which do not use any supporting layer or substrate beneath a catalyst layer.
URI
http://pubs.kist.re.kr/handle/201004/46566
ISSN
19764251
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KIST Publication > Article
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