Stable Organic Field-Effect Transistors for Continuous and Nondestructive Sensing of Chemical and Biologically Relevant Molecules in Aqueous Environment

Title
Stable Organic Field-Effect Transistors for Continuous and Nondestructive Sensing of Chemical and Biologically Relevant Molecules in Aqueous Environment
Authors
Minseong YunAsha SharmaCanek Fuentes-Hernandez황도경Amir DindarSanjeev SinghSangmoo ChoiBernard Kippelen
Keywords
organic field-effect transistor; water-stability; fast chemical detection; reusability
Issue Date
2014-02
Publisher
ACS Applied Materials & Interfaces
Citation
VOL 6, NO 3, 1616-1622
Abstract
The use of organic field-effect transistors (OFETs) as sensors in aqueous media has gained increased attention for environmental monitoring and medical diagnostics. However, stable operation of OFETs in aqueous media is particularly challenging because of electrolytic hydrolysis of water, high ionic conduction through the analyte, and irreversible damage of organic semiconductors when exposed to water. To date, OFET sensors have shown the capability of label-free sensing of various chemical/biological species, but they could only be used once because their operational stability and lifetime while operating in aqueous environments has been poor, and their response times typically slow. Here, we report on OFETs with unprecedented water stability. These OFETs are suitable for the implementation of reusable chemical/biological sensors because they primarily respond to charged species diluted in an aqueous media by rapidly shifting their threshold voltage. These OFET sensors present stable current baselines and saturated signals which are ideal for detection of low concentration of small or large molecules that alter the pH of an aqueous environment. The overall response of these OFET sensors paves the way for the development of continuous chemical/biological nondestructive sensor applications in aqueous media.
URI
http://pubs.kist.re.kr/handle/201004/47390
ISSN
19448244
Appears in Collections:
KIST Publication > Article
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