Charge Transportation at Cascade Energy Structure Interfaces of CuInxGa1-xSeyS2-y/CdS/ZnS for Spontaneous Water Splitting
- Charge Transportation at Cascade Energy Structure Interfaces of CuInxGa1-xSeyS2-y/CdS/ZnS for Spontaneous Water Splitting
- 주오심; 민병권; 황윤정; 채상윤; 박세진
- photoelectrochemical cell; CIGS; CdS; ZnS; Water splitting
- Issue Date
- Electrochimica acta
- VOL 297-640
- A photoelectrode has to generate high enough photovoltage by efficient charge separation spontaneously to split water. In this study, cascade band structures with CdS and ZnS applied to CuInxGa1-xSeyS2-y (CIGS) photoelectrode of water splitting. The morphology, the electronic and the chemical state of CIGS heterojunction films have been characterized by a scanning electron microscopy, X-ray photoelectron spectroscopy, and ultraviolet photoelectron spectroscopy. The CIGS/CdS/ZnS photocathode shows ∼400  mV anodic shift of onset potential and 0.028% efficiency for solar to hydrogen conversion when it couples with a WO3/BiVO4/Co-Pi photoanode for water splitting without external bias potential.
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