Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ
- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ
- 김화진; Carolyn E. Jordan; James H. Crawford; Andreas J. Beyersdorf; Thomas F. Eck; Hannah S. Halliday; Benjamin A. Nault; Lim-Seok Chang; JinSoo Park; Rokjin Park; Gangwoong Lee; Jun-young Ahn; Seogju Cho; Hye Jung Shin; Jae Hong Lee; Jinsang Jung; Deug-Soo Kim; Meehye Lee; Taehyoung Lee; Andrew Whitehill; James Szykman; Melinda K. Schueneman; Pedro Campuzano-Jost; Jose L. Jimenez; Joshua P. DiGangi; Glenn S. Diskin; Bruce E. Anderson; Richard H. Moore; Luke D. Ziemba; Marta A. Fenn; Johnathan W. Hair; Ralph E. Kuehn; Robert E. Holz; Gao Chen; Katherine Travis; Michael Shook; David A. Peterson; Kara D. Lamb; Joshua P. Schwarz
- Issue Date
- Elementa-Science of the Anthropocene : Meteorology and Atmospheric Sciences
- VOL 8, NO 28, 424
- The Korea ？ United States Air Quality Study (May ？ June 2016) deployed instrumented aircraft and ground-based measurements to elucidate causes of poor air quality related to high ozone and aerosol concentrations in South Korea. This work synthesizes data pertaining to aerosols (specifically, particulate matter with aerodynamic diameters <2.5 micrometers, PM2.5) and conditions leading to violations of South Korean air quality standards (24-hr mean PM2.5 < 35 ？g m？3). PM2.5 variability from AirKorea monitors across South Korea is evaluated. Detailed data from the Seoul vicinity are used to interpret factors that contribute to elevated PM2.5. The interplay between meteorology and surface aerosols, contrasting synoptic-scale behavior vs. local influences, is presented. Transboundary transport from upwind sources, vertical mixing and containment of aerosols, and local production of secondary aerosols are discussed. Two meteorological periods are probed for drivers of elevated PM2.5. Clear, dry conditions, with limited transport (Stagnant period), promoted photochemical production of secondary organic aerosol from locally emitted precursors. Cloudy humid conditions fostered rapid heterogeneous secondary inorganic aerosol production from local and transported emissions (Transport/Haze period), likely driven by a positive feedback mechanism where water uptake by aerosols increased gas-to-particle partitioning that increased water uptake. Further, clouds reduced solar insolation, suppressing mixing, exacerbating PM2.5 accumulation in a shallow boundary layer. The combination of factors contributing to enhanced PM2.5 is challenging to model, complicating quantification of contributions to PM2.5 from local versus upwind precursors and production. We recommend co-locating additional continuous measurements at a few AirKorea sites across South Korea to help resolve this and other outstanding questions: carbon monoxide/carb
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