Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ

Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ
김화진Carolyn E. JordanJames H. CrawfordAndreas J. BeyersdorfThomas F. EckHannah S. HallidayBenjamin A. NaultLim-Seok ChangJinSoo ParkRokjin ParkGangwoong LeeJun-young AhnSeogju ChoHye Jung ShinJae Hong LeeJinsang JungDeug-Soo KimMeehye LeeTaehyoung LeeAndrew WhitehillJames SzykmanMelinda K. SchuenemanPedro Campuzano-JostJose L. JimenezJoshua P. DiGangiGlenn S. DiskinBruce E. AndersonRichard H. MooreLuke D. ZiembaMarta A. FennJohnathan W. HairRalph E. KuehnRobert E. HolzGao ChenKatherine TravisMichael ShookDavid A. PetersonKara D. LambJoshua P. Schwarz
Issue Date
Elementa-Science of the Anthropocene : Meteorology and Atmospheric Sciences
VOL 8, NO 28, 424
The Korea ? United States Air Quality Study (May ? June 2016) deployed instrumented aircraft and ground-based measurements to elucidate causes of poor air quality related to high ozone and aerosol concentrations in South Korea. This work synthesizes data pertaining to aerosols (specifically, particulate matter with aerodynamic diameters <2.5 micrometers, PM2.5) and conditions leading to violations of South Korean air quality standards (24-hr mean PM2.5 < 35 ?g m?3). PM2.5 variability from AirKorea monitors across South Korea is evaluated. Detailed data from the Seoul vicinity are used to interpret factors that contribute to elevated PM2.5. The interplay between meteorology and surface aerosols, contrasting synoptic-scale behavior vs. local influences, is presented. Transboundary transport from upwind sources, vertical mixing and containment of aerosols, and local production of secondary aerosols are discussed. Two meteorological periods are probed for drivers of elevated PM2.5. Clear, dry conditions, with limited transport (Stagnant period), promoted photochemical production of secondary organic aerosol from locally emitted precursors. Cloudy humid conditions fostered rapid heterogeneous secondary inorganic aerosol production from local and transported emissions (Transport/Haze period), likely driven by a positive feedback mechanism where water uptake by aerosols increased gas-to-particle partitioning that increased water uptake. Further, clouds reduced solar insolation, suppressing mixing, exacerbating PM2.5 accumulation in a shallow boundary layer. The combination of factors contributing to enhanced PM2.5 is challenging to model, complicating quantification of contributions to PM2.5 from local versus upwind precursors and production. We recommend co-locating additional continuous measurements at a few AirKorea sites across South Korea to help resolve this and other outstanding questions: carbon monoxide/carb
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