Zhang, Kaiqiang Kirlikovali, Kent O. Suh, Jun Min Choi, Ji-Won Jang, Ho Won Varma, Rajender S. Farha, Omar K. Shokouhimehr, Mohammadreza 2024-01-19T17:02:51Z 2024-01-19T17:02:51Z 2021-09-04 2020-07-27 2574-0962 https://pubs.kist.re.kr/handle/201004/118363 Owing to their high theoretical capacity and reliable operational safety, nonaqueous rechargeable aluminum batteries (RABs) have emerged as a promising class of battery materials and been intensively studied in recent years; however, a lack of suitable, high-performing positive electrode materials, along with the need for air-sensitive and expensive ionic liquid electrolytes, has significantly hindered the practical use of RABs in large-scale applications. Therefore, we sought to carefully analyze positive electrode materials and the associated electrolytes that have been reported in these battery systems in order to stimulate the design of the next generation of high-performance and low-cost RABs. In this review, we have summarized the electrode materials that have been used in both nonaqueous and aqueous RAB systems and provided a rational classification based on the types of materials used and their respective structures. Additionally, we have reviewed electrolytes employed in RABs and have categorized them according to two main types of applications, either for fixed battery systems or for use in portable devices. A systematic account of recent developments on RABs, with a focus on electrode materials, innovative perspectives, and impending research efforts on future RABs, has been included. Finally, a proposed liquid RAB system is discussed with the aim of solving issues regarding fast-charging and long operational lifetimes, followed by insights into solid RABs for use in both portable and multistructural RAB systems. English AMER CHEMICAL SOC GRAPHENE OXIDE COMPOSITE VANADIUM CARBIDE MXENE LIQUID-METAL BATTERY CATHODE MATERIAL POSITIVE ELECTRODE HIGH-CAPACITY ENERGY-STORAGE HIGH-VOLTAGE POLYSULFIDE DISSOLUTION POLYMER ELECTROLYTE Recent Advances in Rechargeable Aluminum-Ion Batteries and Considerations for Their Future Progress Article 10.1021/acsaem.0c00957 1 ACS APPLIED ENERGY MATERIALS, v.3, no.7, pp.6019 - 6035 ACS APPLIED ENERGY MATERIALS 3 7 6019 6035 scie scopus 000557375200002 2-s2.0-85089697116 Chemistry, Physical Energy & Fuels Materials Science, Multidisciplinary Chemistry Energy & Fuels Materials Science Review GRAPHENE OXIDE COMPOSITE VANADIUM CARBIDE MXENE LIQUID-METAL BATTERY CATHODE MATERIAL POSITIVE ELECTRODE HIGH-CAPACITY ENERGY-STORAGE HIGH-VOLTAGE POLYSULFIDE DISSOLUTION POLYMER ELECTROLYTE aluminum-ion battery electrode material high performance electrolyte rechargeable