Lee, Eunbyoul Kim, Heejun Choi, Hamin Kim, Se Young Chung, Kyung Yoon 2024-12-06T10:30:26Z 2024-12-06T10:30:26Z 2024-12-06 2024-12 1359-7345 https://pubs.kist.re.kr/handle/201004/151318 We reveal the reversible redox mechanism of Li6PS5Cl in composite cathodes for practical all-solid-state lithium-sulfur batteries. The limited electrochemical reactivity of the non-conducting sulfur-based active material induces the formation of Li6PS5Cl decomposition products, which allows the recrystallization of Li6PS5Cl through a reversible redox process, contributing to the composite cathode capacity. English Royal Society of Chemistry Unraveling the reversible redox mechanism of Li6PS5Cl solid electrolyte in all-solid-state lithium-sulfur batteries Article 10.1039/d4cc04476b 1 Chemical Communications, v.60, no.99, pp.14834 - 14837 Chemical Communications 60 99 14834 14837 N scie scopus 001362151600001 Chemistry, Multidisciplinary Chemistry Article; Early Access