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dc.contributor.authorMoon, Subin-
dc.contributor.authorPark, Young Sun-
dc.contributor.authorLee, Hyungsoo-
dc.contributor.authorJeong, Wooyong-
dc.contributor.authorKwon, Eunji-
dc.contributor.authorLee, Jeongyoub-
dc.contributor.authorYun, Juwon-
dc.contributor.authorLee, Soobin-
dc.contributor.authorKim, Jun Hwan-
dc.contributor.authorYu, Seungho-
dc.contributor.authorMoon, Jooho-
dc.date.accessioned2024-07-18T08:00:54Z-
dc.date.available2024-07-18T08:00:54Z-
dc.date.created2024-07-18-
dc.date.issued2024-08-
dc.identifier.issn1754-5692-
dc.identifier.urihttps://pubs.kist.re.kr/handle/201004/150280-
dc.description.abstractHydrogen peroxide (H2O2) represents a valuable chemical compound and promising energy source due to its high energy density, comparable with that of compressed H-2. However, its production predominantly relies on an energy-intensive process. In this study, we present an efficient strategy for producing H2O2 through a photoelectrochemical (PEC) approach, which involves a 2e(-)-mediated oxygen reduction reaction, integrating Mo-anchored MoOx with a Cu3BiS3-based photocathode. The MoOx-supported Mo improves the adsorption strength of peroxide species and facilitates electron transport, resulting in outstanding activity toward H2O2 production. Consequently, the resulting Cu3BiS3-based photocathode demonstrates significantly enhanced performance, achieving a photocurrent density of 5.21 mA cm(-2) at 0.35 V versus the reversible hydrogen electrode (RHE), a high onset potential of 0.9 V-RHE, and 97% selectivity toward H2O2. Additionally, we successfully implemented an unassisted PEC-PEC coplanar system by coupling a Cu3BiS3-based photocathode with a perovskite-based photoanode, achieving a solar-to-chemical conversion efficiency of 1.46%.-
dc.languageEnglish-
dc.publisherRoyal Society of Chemistry-
dc.titleUnassisted photoelectrochemical hydrogen peroxide production over MoOx-supported Mo on a Cu3BiS3 photocathode-
dc.typeArticle-
dc.identifier.doi10.1039/d4ee00741g-
dc.description.journalClass1-
dc.identifier.bibliographicCitationEnergy & Environmental Science, v.17, no.15, pp.5588 - 5600-
dc.citation.titleEnergy & Environmental Science-
dc.citation.volume17-
dc.citation.number15-
dc.citation.startPage5588-
dc.citation.endPage5600-
dc.description.isOpenAccessN-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.identifier.wosid001265393000001-
dc.identifier.scopusid2-s2.0-85198047147-
dc.relation.journalWebOfScienceCategoryChemistry, Multidisciplinary-
dc.relation.journalWebOfScienceCategoryEnergy & Fuels-
dc.relation.journalWebOfScienceCategoryEngineering, Chemical-
dc.relation.journalWebOfScienceCategoryEnvironmental Sciences-
dc.relation.journalResearchAreaChemistry-
dc.relation.journalResearchAreaEnergy & Fuels-
dc.relation.journalResearchAreaEngineering-
dc.relation.journalResearchAreaEnvironmental Sciences & Ecology-
dc.type.docTypeArticle-
dc.subject.keywordPlusOXYGEN REDUCTION REACTION-
dc.subject.keywordPlusH2O2-
dc.subject.keywordPlusINTERFACE-
dc.subject.keywordPlusSURFACE-
dc.subject.keywordPlusCO-
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KIST Article > 2024
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