Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure

Authors
So, Jae-PilKim, Ha-ReemBaek, HyeonjunJeong, Kwang-YongLee, Hoo-CheolHuh, WoongKim, Yoon SeokWatanabe, KenjiTaniguchi, TakashiKim, JungkilLee, Chul-HoPark, Hong-Gyu
Issue Date
2021-10
Publisher
AMER ASSOC ADVANCEMENT SCIENCE
Citation
SCIENCE ADVANCES, v.7, no.43
Abstract
Quantum confinement in transition metal dichalcogenides (TMDCs) enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic force microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. The emission at the indentation sites exhibits photon antibunching behavior with a g((2))(0) value of similar to 0.3, intensity saturation, and a linearly cross-polarized doublet, at 4 kelvin. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources.
Keywords
LIGHT-EMITTING-DIODES; LOCALIZED EXCITONS; QUANTUM EMITTERS; MONOLAYER; EMISSION; SEMICONDUCTOR; DEFECTS; DOTS
ISSN
2375-2548
URI
https://pubs.kist.re.kr/handle/201004/116286
DOI
10.1126/sciadv.abj3176
Appears in Collections:
KIST Article > 2021
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