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dc.contributor.authorMizuno, N-
dc.contributor.authorSuh, DJ-
dc.contributor.authorHan, W-
dc.contributor.authorKudo, T-
dc.date.accessioned2024-01-21T19:07:22Z-
dc.date.available2024-01-21T19:07:22Z-
dc.date.created2022-01-11-
dc.date.issued1996-12-23-
dc.identifier.issn1381-1169-
dc.identifier.urihttps://pubs.kist.re.kr/handle/201004/144196-
dc.description.abstractKeggin-type 12-molybdophosphates have been found to catalyze the selective oxidation of isobutane, propane, and ethane into methacrylic acid, acrylic acid, and ethene, respectively, with molecular oxygen. Cs+-, Fe3+-, or Ni2+-substitution for H+ and V5+-substitution for Mo6+ in H3PMo12O40 enhanced the catalytic activity for the oxidation of propane. Among the catalysts tested Cs2.5Fe0.08H1.26PVMo11O40 gave the highest yield of acrylic acid: 13%. It was suggested by IR, XRD, TG-DTA data that the Keggin structure was maintained during the oxidation.-
dc.languageEnglish-
dc.publisherELSEVIER SCIENCE BV-
dc.subjectBUTANE SELECTIVE OXIDATION-
dc.subjectHETEROPOLY COMPOUNDS-
dc.subjectMETHACRYLIC-ACID-
dc.subjectACRYLIC-ACID-
dc.subject12-MOLYBDOPHOSPHORIC ACID-
dc.subjectPROPANE-
dc.subjectISOBUTANE-
dc.subjectOXYGEN-
dc.subjectPHASE-
dc.subjectAMMOXIDATION-
dc.titleCatalytic performance of Cs2.5Fe0.08H1.26PVMo11O40 for direct oxidation of lower alkanes-
dc.typeArticle-
dc.identifier.doi10.1016/S1381-1169(96)00332-9-
dc.description.journalClass1-
dc.identifier.bibliographicCitationJOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, v.114, no.1-3, pp.309 - 317-
dc.citation.titleJOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL-
dc.citation.volume114-
dc.citation.number1-3-
dc.citation.startPage309-
dc.citation.endPage317-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.identifier.wosidA1996WC26500032-
dc.identifier.scopusid2-s2.0-0030599598-
dc.relation.journalWebOfScienceCategoryChemistry, Physical-
dc.relation.journalResearchAreaChemistry-
dc.type.docTypeArticle-
dc.subject.keywordPlusBUTANE SELECTIVE OXIDATION-
dc.subject.keywordPlusHETEROPOLY COMPOUNDS-
dc.subject.keywordPlusMETHACRYLIC-ACID-
dc.subject.keywordPlusACRYLIC-ACID-
dc.subject.keywordPlus12-MOLYBDOPHOSPHORIC ACID-
dc.subject.keywordPlusPROPANE-
dc.subject.keywordPlusISOBUTANE-
dc.subject.keywordPlusOXYGEN-
dc.subject.keywordPlusPHASE-
dc.subject.keywordPlusAMMOXIDATION-
dc.subject.keywordAuthorlower alkanes-
dc.subject.keywordAuthoroxidation-
dc.subject.keywordAuthorheteropoly compounds-
dc.subject.keywordAuthoriron-
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